Claudio U. Hail, Lior Michaeli, Harry A. Atwater
Abstract
Achieving spatiotemporal control of light at subwavelength and subcycle scales is an important milestone in the development of new photonic materials and technologies. Ultrafast spatiotemporal light modulation currently relies on electronic interband and intraband transitions that yield pronounced refractive index changes but typically suffer from slow, picosecond response times due to carrier relaxation. Here we show that by leveraging resonant light-matter interactions in a high-quality factor metasurface it is possible to use the optical Kerr effect, a weaker, but instantaneous optoelectronic polarization effect, to achieve ultrafast, reconfigurable light modulation with unprecedented spatial and temporal control. By the subwavelength all-optical tuning of the refractive index of the dielectric metasurface unit cells, we experimentally demonstrate pulse-limited beam steering with a 74-fs response time at angles up to 13° in the near-infrared. The steering originates from the Kerr effect with a background contribution arising from slower two-photon-excited free carrier absorption. Additionally, we observe spatial back-action, linear frequency conversion, and demonstrate arbitrary ultrafast spatial light modulation in two dimensions. Our findings open the possibility of realizing new ultrafast physics in metastructures with applications in signal processing, pulse shaping, and ultrafast imaging.